THESIS
2018
xv, 44 pages : illustrations (chiefly color) ; 30 cm
Abstract
The enhanced superconductivity in few layer 2H-TaS
2 and suppressed CDW transition of
nanoribbon 1T-TaS
2 have been investigated in this thesis.
Transport properties of different thickness 2H-TaS
2 reveal the suppression of CDW transition
signature in 2D region. Further, the electron dominant carrier density in the order of 10
22 ? ∙
??
−3 manifests its metallic behavior. Superconductivity in atomically thin 2H-TaS
2 is strongly
enhanced, the critical temperature of a trilayer sample can be up to 2.6 K compared with 0.8 K
in bulk crystals. Four-probe differential resistance method measured superconducting gap fits
well with BCS model. The enhanced superconductivity may be a consequence of suppression
of CDW transition and the enhancement of DOS at Fermi level.
Moreover, the transport...[
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The enhanced superconductivity in few layer 2H-TaS
2 and suppressed CDW transition of
nanoribbon 1T-TaS
2 have been investigated in this thesis.
Transport properties of different thickness 2H-TaS
2 reveal the suppression of CDW transition
signature in 2D region. Further, the electron dominant carrier density in the order of 10
22 ? ∙
??
−3 manifests its metallic behavior. Superconductivity in atomically thin 2H-TaS
2 is strongly
enhanced, the critical temperature of a trilayer sample can be up to 2.6 K compared with 0.8 K
in bulk crystals. Four-probe differential resistance method measured superconducting gap fits
well with BCS model. The enhanced superconductivity may be a consequence of suppression
of CDW transition and the enhancement of DOS at Fermi level.
Moreover, the transport characterization of bulk crystal 1T- TaS
2 demonstrates its unique
three CDW evolutions with temperature. After eliminating the disturbances from measurements,
the RIE etched decreased width nanoribbon like channels behave similar to the decreased
thickness samples, showing a suppressed CDW transition signature. And when the width of
channel still goes down, the CDW transition order will be concealed. To explain this trend, we
proposed a free energy theory indicating that the decreased width will introduce higher and
more stable barrier between CDW transitions. Our results establish that the decreased x or y-axis
of 1T- TaS
2 will also strongly affect the CDW order.
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